Jeong, S., Choi, M., Jagdale, G., Zhong, Y., Siepser, N., Wang, Y., Zhan, X., Baker, L.^‡, Ye, X.^‡ Unraveling Structural Sensitivity of CO2 Electroreduction at Facet-Defined Nanocrystal via Correlative Single-Entity and Macroelectrode Measurements. J. Am. Chem. Soc. 2022, 144, 12673-12680. DOI: 10.1021/jacs.2c02001 Highlighted by JACS Spotlights.